Darsteller
- Oyiza Momoh
- Aneisha Jones
- Sam Strike
- Dan Morgan
- Oscar Jacques
- Tom Tupper
- Natasha Watson
- Z.0.E.
- Rachel Petladwala
- Rose Gupta
- Ben Kerfoot
- Oscar Cole
- Charlene Osuagwu
- Carrie Stewart
- Jonny Freeman
- Frank London
- Moustafa Chousein-Oglou
- Blane Whittaker
- Bel Powley
- Daisy Millar
- Danny John-Jules
- Lenny Bicknall
- Julian Bleach
- Grandmaster
- Kerry Shale
- Voice of the Grand Master
Staffel 1
- Winnie Mromria
- Voice of the Grand Master
Staffel 2
- Moya Brady
- Professor Sally Moreau
The Guinea Pig (S.K.U.L. Evil Scientist)
- Steve Furst
- Tony Frisco
(S.K.U.L. – Crush’s Manager)
- Julian Gregory
- „Crush“
- Ryan Gregory
- „Crush“
- Eliot Gregory
- „Crush“
- Siobhan Hewlett
- Sony Frost
S.K.U.L. Secretary and ex-TV Weather Girl
- Angus Barnett
- Brent Gilbert
S.K.U.L. Retired Tour Guide
- Steven Meiklejohn
- The Worm
S.K.U.L. Hacker
- Toby Regbo
- Chad Turner
S.K.U.L. and CIA Double Agent
- Jeremy Swift
- Silas Fenton
Aspiring S.K.U.L. Agent and Inventor
- Rula Lenska
- Vanessa Zietgeist
S.K.U.L. Beautician
- Alex Ferns
- General Ryan Scarp
S.K.U.L. and British Army General
- Rebecca Palmer
- Carla Terrini
M.I.9, S.K.U.L. – Air One Agent
- Mark Bagnell
- Agent Zero
The Grand Master’s Nephew
- Christopher Stanton
- Mr. Kenneth Flatley
Direktor von Saint Hope
- Scott Gibbins
- Stewart Critchley
- Jane Cameron
- Ms. Templeman
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